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Modeling of Time-Resolved Spectra |
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Katharine M. Mullen, Ivo H.M. van Stokkum A PSE for hierarchical modeling
of time-resolved spectra
Lay report, lekenverslag (in Dutch) Application of Global and Target Analysis
in Photobiophysics
Global and Target Analysis of spectroscopic
data, in particular time resolved spectra, play a central role in Photobiophysics. Applications are
in the primary charge transfer steps in the reaction centers of purple
bacteria and green plants, energy transfer in antennae (in particular
LHC-II), Stark spectroscopy, blue-light photoreceptors (in particular flavoproteins), carotenoid-chlorophyll
complexes (like PCP and FCP), Green Fluorescent Protein, and secondary
structure changes in proteins. The streak scope project (financially
supported by SLW and our faculty), is now routinely producing high quality
emission data, with the desired (sub)picosecond
time resolution. Corrections for instrumental curvature and drift have been
implemented, and the global analysis of the high quality data furnishes
publishable results. Collaborations
(dr. A.M. Brouwer,
prof.dr. Wybren Jan Buma,
prof.dr. K.J. Hellingwerf, dr.
R.M. Williams ) Wageningen Agricultural University
(prof.dr. H. van Amerongen,
prof.dr. A.J.W.G. Visser ) International
dr. Delmar S. Larsen |
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